Journal
NANO RESEARCH
Volume 8, Issue 11, Pages 3472-3479Publisher
TSINGHUA UNIV PRESS
DOI: 10.1007/s12274-015-0845-4
Keywords
hydrogen storage; metal-organic frameworks; nitrogen-doped porous carbon; hydrazine
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Funding
- National Natural Science Foundation of China [21201134, 21571145]
- Natural Science Foundation of Jiangsu Province [BK20130370]
- Natural Science Foundation of Hubei Province [2013CFB288]
- Creative Research Groups of Hubei Province [2014CFA007]
- Large-scale Instrument and Equipment Sharing Foundation of Wuhan University
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Well-dispersed bimetallic NiRh nanoparticles (NPs) with different compositions supported on nitrogen-doped porous carbon (NPC) derived from metal-organic frameworks (ZIF-8) were synthesized through a co-reduction method. The NPC-900 supported NiRh catalyst exhibits the highest catalytic activity and 100% hydrogen selectivity toward hydrogen generation from hydrazine. These properties might be attributed to the high surface area and high graphitization of the NPC. This strategy may open up a new avenue for designing high-performance catalysts by utilizing NPC as a support to anchor active metal NPs for additional applications.
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