Journal
ISRAEL JOURNAL OF CHEMISTRY
Volume 51, Issue 2, Pages 238-246Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ijch.201100021
Keywords
catalyst stability; multi-electron redox processes; polyoxometalate; water oxidation catalyst; water splitting
Categories
Funding
- US Department of Energy [DE-FG02-03ER15461]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [0958205] Funding Source: National Science Foundation
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Water oxidation catalysts (WOCs) are of core importance in several green energy production technologies, including water splitting and water reduction of CO2 driven by electrochemical potential and/or photons (radiant energy). General challenges in solar fuel generating structures, WOC design concepts, and some success-limiting considerations in WOC development are described. The first class of WOCs are presented that combine the stability benefits of heterogeneous WOCs with the reactivity and other benefits of homogeneous WOCs.
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