Journal
INORGANIC CHEMISTRY
Volume 53, Issue 14, Pages 7086-7088Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ic5012764
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Funding
- National Science Foundation of China [21271117, 21371179]
- Shandong Natural Science Fund for Distinguished Young Scholars [JQ201003]
- National Science Foundation of Shandong Province [BS2011CL041]
- Fundamental Research Funds for the Central Universities [13CX05010A, 13CX02006A]
- [NCET-11-0309]
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A new porous zirconium metal organic framework (Zr MOF), Zr-6(mu(3)-O)(4)(mu 3OH)(4)(OH)(6)(H2O)(6)(BTB)(2)center dot 6DMF center dot H2O (1; H3BTB = 5'-(4-carboxyphenyl) [1,1':3',1 ''-terphenyI]-4,4 ''-dicarboxylic acid), based on Zr-6 clusters and tricarboxylate ligands has been constructed and characterized. The Zr-6 clusters were linked by BTB ligands to generate a 2D network of kgd topology. The interpenetrations among the 2D networks gave rise to a 3D porous framework, which represents the first Zr MOF constructed from 2D -> 3D interpenetration. The gas uptake and catalytic properties for 1 have also been studied.
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