Journal
INORGANIC CHEMISTRY
Volume 53, Issue 7, Pages 3392-3403Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ic402798f
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Funding
- Centre National de la Recherche Scientifique (ICMUB) [UMR CNRS 6302]
- CNRS
- Universite de Bourgogne
- Conseil Regional de Bourgogne through the 3MIM integrated project (Marquage de Molecules par les Metaux pour l'Imagerie Medicate)
- French Ministry of Research
- Agence Nationale de la Recherche (ANR)
- Sciences and Engineering Research Council of Canada (NSERC)
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Red (no styryl), green (monostyryl), and blue (distyryl) BODIPY-gallium(III) (BODIPY = boron-dipyrromethene) corrole dyads have been prepared in high yields using click chemistry, and their photophysical properties are reported. An original and efficient control of the direction of the singlet energy transfers is reported, going either from BODIPY to the gallium-corrole units or from gallium-corroles to BODIPY, depending upon the nature of the substitution on BODIPY. In one case (green), both directions are possible. The mechanism for the energy transfers is interpreted by means of through-space Forster resonance energy transfer (FRET).
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