Journal
INORGANIC CHEMISTRY
Volume 47, Issue 22, Pages 10217-10219Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ic8014892
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Funding
- Chuo University
- Inamori Foundation
- Tokuyama Science Foundation
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Chemically induced longitudinal contraction of the square-antiprism coordination polyhedron of a peripherically substituted bis(phthalocyaninato)dysprosiumate(III), a dysprosium-based single-4f-ionic single-molecule magnet having a J(Z) = +/- 13/2 Kramers doublet ground state, resulted in drastic changes in dynamical magnetism including a doubling of the energy barrier, a 2-order-of-magnitude decrease of the spin reversal rate, a significant rise of the blocking temperature, and the first observation of the emergence of a large remanent magnetization.
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