Journal
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Volume 57, Issue 39, Pages 13019-13025Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.iecr.8b02036
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Funding
- NSFC [51702284]
- Startup Foundation for Hundred-Talent Program of Zhejiang University [112100-193820101/001/022]
- Fundamental Research Funds for the Central Universities [112109*172210171]
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Development of high performance anode materials is of critical importance for advanced lithium-ion batteries. Herein, we report a novel 3D hybrid composed of well-dispersed Co2P nanoparticles embedded in N-doped carbon nanotubes grown on porous carbon polyhedral (Co2P/NCNTFs) as advanced electrode for lithium-ion batteries. The Co2P/NCNTF electrode is synthesized with a facile pyrolysis and phosphidation method derived from a cobalt-based zeolitic imidazolate framework. The resultant Co2P/NCNTFs hybrid demonstrates superior electrochemical performance in lithium-ion batteries, with a large discharge capacity of 906 mA h g(-1) at 100 mA g(-1), excellent rate performance of 508 mA h g(-1) at 6.4 A g(-1), high Coulombic efficiency of 99.4% after 300 cycles at 100 mA g(-1), and high cycling performance with a capacity retention of 94.7%, which is among the best obtained results for Co2P-based anode materials.
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