Journal
HELVETICA CHIMICA ACTA
Volume 97, Issue 1, Pages 128-136Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/hlca.201300296
Keywords
Subergorgia suberosa; Lactones; Metabolites; Suberosanones A-C; Corals
Categories
Funding
- National Marine '863' Project [2013AA092902]
- National Natural Science Fund [21172094]
- Guangdong Technology Project [2011A08050407]
- Tianhe Technology Project [2006Z3-E4041]
- Biotechnology Research Institute at the Hong Kong University of Science and Technology
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Two unusual novel bicyclic lactones, suberosanones A and B (1 and 2, resp.), characterized by the co-occurrence of cyclopentenone and butanolide rings within the same molecule, along with one tricyclic cyclopentenone derivative, suberosanone C (3), were isolated from the South China Sea gorgonian coral Subergorgia suberosa. Their structures were unambiguously established by detailed spectroscopic analyses (NMR, IR, and HR-MS). The absolute configurations of 1 and 2 were determined by quantum-chemical calculations using the time-dependent density-functional theory (TDDFT) method. All compounds showed neither antifouling activity against Balanus amphitrite larvae settlement nor antibacterial activity against a panel of bacterial strains at concentrations up to 25 mu g/ml.
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