Journal
HELVETICA CHIMICA ACTA
Volume 91, Issue 11, Pages 2181-2202Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/hlca.200890236
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The A*[s]U-(*) dinucleosides 1 and 2 form thermoreversible gels in organic solvents. The basis of the gelation is the formation of linear aggregates by base pairing following desolvation of the nucleobases. This is evidenced by the absence of gel formation by the C(6)-deaminated analogue 3 of 1, the correlation of gelation with the anti-conformation, as preferred for 1, and the temperature-, concentration-, and time-dependent CD spectra. The gels were also characterized by the minimum gelation concentration, the gel-sol transition (melting) temperature and rheological properties.
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