4.7 Article

A high-power ultrasonic microreactor and its application in gas-liquid mass transfer intensification

Journal

LAB ON A CHIP
Volume 15, Issue 4, Pages 1145-1152

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c4lc01431f

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Funding

  1. National Natural Science Foundation of China [21225627, 91334201]
  2. Ministry of Science and Technology of China [2012BAA08B02]

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The combination of ultrasound and microreactor is an emerging and promising area, but the report of designing high-power ultrasonic microreactor (USMR) is still limited. This work presents a robust, high-power and highly efficient USMR by directly coupling a microreactor plate with a Langevin-type transducer. The USMR is designed as a longitudinal half wavelength resonator, for which the antinode plane of the highest sound intensity is located at the microreactor. According to one dimension design theory, numerical simulation and impedance analysis, a USMR with a maximum power of 100 W and a resonance frequency of 20 kHz was built. The strong and uniform sound field in the USMR was then applied to intensify gas-liquid mass transfer of slug flow in a microfluidic channel. Non-inertial cavitation with multiple surface wave oscillation was excited on the slug bubbles, enhancing the overall mass transfer coefficient by 3.3-5.7 times.

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